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政大機構典藏 > 理學院 > 應用物理研究所 > 期刊論文 > Item 140.119/70492

Please use this identifier to cite or link to this item: https://nccur.lib.nccu.edu.tw/handle/140.119/70492

Title:	Magnetic correlations in HoxTb2−xTi2O7
Authors:	陳洋元 L. J. Chang;W. Schweika;Kao,Y. -J.;Chou,Y. Z.;J. Perßon;Chen,Y. Y.
Contributors:	應物所
Date:	2011
Issue Date:	2014-10-09 15:48:26 (UTC+8)
Abstract:	Polycrystalline samples of HoxTb2−xTi2O7 (0 < x < 2) have been prepared and characterized for their structural and magnetic properties. The parent compounds of this solid solution are the spin ice Ho2Ti2O7 and the spin liquid Tb2Ti2O7. Specific-heat measurements on HoTbTi2O7 (x = 1.0) reveal the absence of a long-range order state above 0.5 K. The integrated entropies of all HoxTb2−xTi2O7 specimens up to 30 K scale well with the ratio of spin ice and spin liquid in the composition. The neutron diffraction spectrum of HoTbTi2O7 exhibits a dipolar spin-ice pattern and can be well described by mean-field theory for 111 Ising spins, nearest-neighbor exchange, and dipolar interactions. Inelastic neutron scattering on HoTbTi2O7 reveals two dispersionless excitations, one of ∼2.5 meV out of the ground state, and a 4-meV transition out of an excited state. We argue that these data suggest that the very strong single-ion effects of Ho2Ti2O7 and Tb2Ti2O7 persist in the HoxTb2−xTi2O7(0 < x < 2) solid solution, whereas the Tb-Ho correlations are weak, resulting in small shifts in the energy scales but with no dramatic effect on the bulk properties.
Relation:	Physical review. B,83(14),144413
Data Type:	article
DOI 連結:	http://dx.doi.org/10.1103/PhysRevB.83.144413
DOI:	10.1103/PhysRevB.83.144413
Appears in Collections:	[應用物理研究所 ] 期刊論文

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